Low spatial frequency laser-induced periodic surface structures in fused silica inscribed by widely tunable femtosecond laser pulses

Abstract

The formation and evolution of laser-induced periodic surface structures in fused silica under irradiation of widely tunable (in the 1–3 upmum range) linearly polarized femtosecond (200 fs) pulses was studied experimentally. The structures were inscribed in high fluence regime (exceeding the surface ablation threshold for a single pulse) and characterized by using scanning electron microscopy and two dimensional Fourier transform. The results revealed rapid (after irradiation with a few successive pulses) formation of periodic laser-induced periodic surface structures aligned parallel to laser polarization, whose period increases with increasing the inscription wavelength, obeying the lambda /n law. With further increase of number of pulses, the generated structures gradually reorganize into laser polarization-independent low spatial frequency annular structures associated with formation of the damage crater, which fully established after irradiation with a few tens of successive laser pulses. This particular evolution scenario was observed over the entire wavelength tuning range of incident pulses.