Abstract

Monocrystalline Mg-Al-O barriers for magnetic tunnel junctions (MTJs) were fabricated by natural oxidation of Mg-Al thin films. The naturally oxidized Mg-Al-O barrier had a cation-disorder MgAl2O4 structure, and Fe/Mg-Al-O/Fe(001) MTJs showed a tunnel magnetoresistance (TMR) ratio of over 180% at room temperature. In addition, the natural oxidation process resulted in tunnel barriers with a resistance area product (RA) of less than 5 Ω·μm2. We observed clear magnetization switching in a CoFe/Mg-Al-O/CoFe MTJ by spin-transfer torque. These results indicate that the natural oxidation of Mg-Al alloy is an effective method for processing cation-disorder MgAl2O4 barrier for coherent TMR with low RA.

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