Abstract

Two techniques are employed to probe the low frequency modes observed in specific heat measurements of amorphous semiconducttors. A disorder induced coupling of acoustic modes to optical radiation in these materials is demonstrated by the experimental observation of a far infrared and microwave absorption whose magnitude correlates with the density of states inferred from the T3 term in the low temperature specific heat. Enhanced densities of low frequency modes, which contribute to the T term of specific heat in glassy As2S3 and As2Se3, are confirmed from As75 spin-lattice relaxation rates determined by pulsed nuclear quadrupole resonance (NQR).

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