Abstract

The pairing mechanism of high-temperature superconductivity in cuprates is regarded as one of the most challenging issues in condensed matter physics. The core issue concerns how the Cooper pairs are formed. Here we report spin-resolved tunneling measurements on extremely underdoped Bi2Sr2−xLaxCuO6+δ. Our data reveal that, when holes are doped into the system, the antiferromagnetic order is destroyed, while at the same time an increasing density of states (DOS) peaked at around 200 meV appears within the charge transfer gap. Meanwhile, an electronic structure with 4a0 × 4a0 basic plaquettes emerges inhomogeneously, with an area fraction that grows with hole doping. In each plaquette, there are some unidirectional bars (along the Cu-O bond) which are most pronounced at energies near peaks in the DOS around at 25 meV, with an intensity that is especially pronounced at oxygen sites. We argue that the atomically resolved low-energy DOS and related gap are closely associated with some kinds of density waves, possibly reflecting modulations of the electron density, or a pair-density wave, i.e. a modulation of the local pairing. Our work sheds new light on the doping induced electronic evolution from the “parent” insulator of the cuprate superconductors.

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