Long-term spatiotemporal variation in atmospheric aerosol properties over Türkiye based on MERRA-2 reanalysis data: aerosol classification based on city type.

Abstract

Due to their complex aerosol characteristics, it is crucial to analyze the trends and properties of atmospheric aerosols over the eastern Mediterranean countries. This study comprehensively evaluates Aerosol Optical Depth (AOD) and Angström Exponent (AE) trends and aerosol classification over Türkiye, using the MERRA-2 reanalysis data from 1980 to 2019. The spatial distributions of AOD and AE were determined across various temporal scales, including multiannual, 5-year intervals, seasonal, and monthly periods. The analysis of the spatial distribution of AOD values revealed that the mean values in the northwestern areas, ranging from 0.20 to 0.25, were comparatively higher than those observed in the eastern regions, which ranged from 0.10 to 0.15. Between 1980 and 1994, the AOD values gradually increased, followed by a subsequent decline from 1995 to 2019. Based on 5-year intervals between 1980 and 2019, the coastal regions exhibited higher AOD values than the inland areas. Specifically, higher AOD values were noted between May and August, whereas lower values were observed during autumn and winter. Additionally, higher AE values were detected over the northwestern region, while the southeastern region had the lowest AE values, particularly during spring, attributed to the frequent occurrence of dust transport events in this area. The AOD and AE values were also examined in different city types, using the population thresholds of the European Commission. The global city category consisting only of Istanbul showed the highest AOD values across all seasons, while the category of very small cities, which includes 12 cities, had the lowest AOD values. Furthermore, this study investigated the contributions of dominant aerosol categories across various city types based on multiannual and seasonal variations of AOD and AE. The results showed that mixed and continental aerosols had higher portions across all city types. However, biomass burning/industrial and mixed aerosol categories were more prominent in global and large cities. Overall, this study provides a comprehensive overview of the atmospheric aerosol properties in Türkiye and can serve as a useful guide for researchers intending to conduct future studies utilizing AOD and AE data obtained through MERRA-2 aerosol diagnosis.