Abstract

Since the 1970s, air quality has improved at the national level in the United States, coincident with the introduction of the Clean Air Act and other air pollution regulations at a greater frequency. We present a case study from Philadelphia, Pennsylvania—the sixth most populous city in the United States. The main objectives of this study are to analyze long-term trends of particulate matter (PM) from 1986 to 2021 in Philadelphia and to examine their association with the introduction of environmental policies relevant to air pollution at the federal, state, and local levels. We find that annual PM10 concentration decreased by 47% from 1986 to 2021 and annual PM2.5 concentration decreased by 31% from 2000 to 2021 in Philadelphia. We find that carbonaceous content (both elemental and organic carbon) has declined over the same period of 2000 to 2021, demonstrating its contribution to overall PM2.5 reduction in Philadelphia. In Philadelphia, high PM concentrations occur in the summer months; however, seasonal patterns have changed for PM10 in the last decade (2011–2020). Overall, PM reductions occurred over all seasons, with the greatest reductions occurring for PM2.5 during summer months and for PM10 during winter months. The Clean Air Act contributed to the creation of many regulatory policies that address unhealthy levels of PM. The introduction of various environmental policies that target the transportation sector has contributed to the reduction of PM levels in Philadelphia. Air quality would continue being improved by implementing such environmental policies specific to the emissions sectors.

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