Abstract
Dynamic deformation and absorbing regulation are still challenging for designing lightweight and high-efficiency microwave absorbing materials, which are of great indispensability to satisfy changeable and complex electromagnetic environments. Herein, a compressible composite foam with sea-island structure was prepared by loading porous polyaniline (PANI)/Ti3C2Tx composites on ethylene/vinyl acetate (EVA) skeleton via a thermally induced phase separation strategy. The composite foam exhibits a minimum reflection loss (RLmin) of −57.84 dB and an effective absorption bandwidth (EAB, RL ≤ −10 dB) of 1.86 GHz (8.2–10.05 GHz) at 3.4 mm. Notably, the microwave absorption (MA) performance can be precisely regulated by simply adjusting the compression ratio of composite foam. The RL peaks shift towards higher frequencies with increasing compression ratios, originating from changes in the internal conductive network. Even under 30 % compression strain, the composite foam still maintains RLmin of −21.53 dB and broadens EAB up to 2.71 GHz at 2.0 mm. This combination of compression capabilities and dynamically tunable MA performance may expand a novel approach to designing multifunctional polymer-based foam.
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