Abstract
We synthesized a novel phenanthroline-based mononuclear Fe(II) compound [Fe(TTD)2(NCS)2]⋅CH3CN (1, TTD = 1,4,8,9-tetraaza-triphenylene-2,3-dicarbonitrile). And its crystal structure, optical and magnetic properties were analyzed. The thermally induced SCO of the compound is a one-step abrupt transition. In addition, light can also control the spin state of the compound. By using 660 nm light-excited compound, LIESST (light-induced excited spin-state trapping) effect can be achieved.
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