Abstract
Various kinetic parameters of the KrF excimer generated by the use of photoassociative pumping have been measured under simple and controllable conditions. The population transfer rate coefficient between the B2Σ+ and C2Π states has been directly determined to be (1.2±0.3)×10-10 cm3/s for Kr buffer gas. The radiative lifetime of the C2Π state and the quenching rate coefficients for F2 and Kr gases are also given as 60±10 ns, (2.5±1)×10-10 cm3/s, and (7±3)×10-12 cm3/s, respectively.
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