Abstract

The bandgap dependence on the number of atomic layers of some families of two-dimensional (2D) materials can be exploited to engineer and use lateral heterostructures (LHs) as high-performance field-effect transistors (FETs). This option can provide very good lattice matching as well as high heterointerface quality. More importantly, this bandgap modulation with layer stacking can give rise to steep transitions in the density of states (DOS) of the 2D material that can eventually be used to achieve sub-60 mV/decade subthreshold swing in LH-FETs thanks to an energy-filtering source. We have observed this effect in the case of a PdS2 LH-FET due to the particular DOS of its bilayer configuration. Our results are based on ab initio and multiscale materials and device modeling and incite the exploration of the 2D-material design space in order to find more abrupt DOS transitions and better suitable candidates.

Highlights

  • The bandgap dependence on the number of atomic layers of some families of two-dimensional (2D) materials can be exploited to engineer and use lateral heterostructures (LHs) as high-performance field-effect transistors (FETs)

  • In this work we investigate the potential of noble transition-metal dichalcogenides (TMDs) as channel materials for LH-FETs, showing the possibility to engineer an energy-filtering source in order to obtain sub-60 mV/dec subthreshold swing (SS) at room temperature and to design devices with competitive figures of merit when compared to the predictions of the International Roadmap for Devices and Systems (IRDS).[29]

  • We have shown that the strong dependence of the bandgap upon the number of layers of noble TMDs can be used to devise electron devices based on transport through lateral heterostructures of TMDs, such as LH-FETs and LH-resonant tunneling diode (RTD)

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Summary

Introduction

The bandgap dependence on the number of atomic layers of some families of two-dimensional (2D) materials can be exploited to engineer and use lateral heterostructures (LHs) as high-performance field-effect transistors (FETs). This option can provide very good lattice matching as well as high heterointerface quality. This bandgap modulation with layer stacking can give rise to steep transitions in the density of states (DOS) of the 2D material that can eventually be used to achieve sub-60 mV/decade subthreshold swing in LH-FETs thanks to an energy-filtering source. FETs made of few-layer PdSe2 and PtSe2 have been experimentally realized showing ambipolar transfer characteristics,[13,19,20] and a large dependence of PtSe2 conductance on the number of layers has been observed.[13]

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