Abstract
Results are described for experiments on the effect of selective translational, rotational, vibrational, and electronic excitation of reactants in bimolecular reactions using flow systems, crossed molecular beams, UV- and IR-laser excitation, and reactant and product detection by time-resolved atomic line resonance absorption, mass spectrometry, LIF, and CARS. The experimental results are compared with the results of quantum and quasiclassical trajectory studies on ab initio potential surfaces and with thermal rate parameters. 85 references, 16 figures, 1 table.
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