Abstract

This paper presents a detailed investigation of the motion of individual micro-particles in a moderately-viscous liquid in direct response to a local, laser-induced temperature gradient. By measuring particle trajectories in 3D, and comparing them to a simulated temperature profile, it is confirmed that the thermally-induced particle motion is the direct result of thermophoresis. The elevated viscosity of the liquid provides for substantial differences in the behavior predicted by various models of thermophoresis, which in turn allows measured data to be most appropriately matched to a model proposed by Brenner. This model is then used to predict the effective force resulting from thermophoresis in an optical trap. Based on these results, we predict when thermophoresis will strongly inhibit the ability of radiation pressure to trap nano-scale particles. The model also predicts that the thermophoretic force scales linearly with the viscosity of the liquid, such that choice of liquid plays a key role in the relative strength of the thermophoretic and radiation forces.

Highlights

  • We predict when thermophoresis will strongly inhibit the ability of radiation pressure to trap nano-scale particles

  • The model predicts that the thermophoretic force scales linearly with the viscosity of the liquid, such that choice of liquid plays a key role in the relative strength of the thermophoretic and radiation forces

  • It has long been known that particles immersed in a gas or liquid will migrate in response to a thermal gradient, an effect known as thermophoresis

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Summary

TITLE AND SUBTITLE

U.S Naval Research Laboratory, 4555,Optical Sciences Division,4555 Overlook Avenue, SW,Washington,DC,20375.

14. ABSTRACT
18. NUMBER OF PAGES
Introduction
Experiment
Analysis
Radiation pressure
Thermophoresis
Transfer of optical momentum to the liquid
Discussion
The McNab-Meisen model
The Schimpf-Semenov dipole-dipole model
The Ruckenstein model
The Duhr-Braun ionic-shielding model
The Brenner model
Extension to small particles in an optical trap
Findings
R3 c np2 nl 2 n
Conclusion
Full Text
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