Abstract
The state population distributions of the nascent products for Ca+NF3 -> CaF+NF2 and Ca+CHF3 -> CaF+CHF2 reactions were studied by means of LIF in a beam-gas arrangement. From the LIF spectra of CaF and the computer simulations, the CaF vibrational distributions for both reactions were found to be similar to the Boltzmann distribution and the internal energy disposal of CaF was determined quantitatively. The results of the spectral simulation and the information theory computation indicate that NF2 and CHF2 radicals were vibrationally and rotationally excited. These tow reactions are thought to be direct collision reactions with the late exoeergicity on potential surface.
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