Abstract
Resonance fluorescence series in the B 1Π- X 1Σ + band system of the isotopic lithium hydrides were observed for the first time. Six series of 7LiD and eight of 6LiH were excited by a frequency-doubled dye laser pumped by a frequency-doubled YAG laser. These observations have provided experimental data to compare with previous theoretical transition probabilities (W. T. Zemke, K. R. Way, and W. C. Stawalley, J. Chem. Phys. 69, 402–408 (1978)). Excellent correspondences between the observed fluorescence intensities and the theoretical results have been realized.
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