Abstract

We report a study on the heat transport of an S = 1 Haldane chain compound Ni(C3H10N2)2NO2ClO4 at low temperatures and in magnetic fields. The zero-field thermal conductivities show a remarkable anisotropy for the heat current along the spin-chain direction (κb) and the vertical direction (κc), implying a magnetic contribution to the heat transport along the spin-chain direction. The magnetic-field-induced change of the spin spectrum has obviously opposite impacts on κb and κc. In particular, κb(H) and κc(H) curves show peak-like increases and dip-like decreases, respectively, at ∼9 T, which is the critical field that minimizes the spin gap. These results indicate a large magnetic thermal transport in this material.

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