Abstract

In order to acquire a soft magnetic film with low conductivity and large magnetic anisotropy, the strain-modulated magnetic anisotropy is studied in epitaxial MgFe2O4 (MFO) films. The MFO films with thicknesses of 25, 48, 75, and 110 nm are grown on the MgAl2O4 (MAO) (100) substrate using a pulsed laser deposition technique. Due to the large lattice-mismatch (3.34%) between MFO and MAO substrates, the interface exhibits a large tetragonal compressive strain. The results of field-dependent magnetization suggest the soft magnetic nature of all the measured MFO films. The analysis of angular dependent ferromagnetic resonance reveals the large uniaxial magnetic anisotropy energy (Ku) of −1.62 × 106 erg/cm3 in the highly strained 25 nm film, and Ku decreases with the increasing thickness due to strain relaxation. The observed large magnetic anisotropy in these highly strained MFO thin films is larger than most of the soft ferrite thin films, which arise due to tetragonal distortion and inverse magnetostriction. The epitaxial MFO thin films with enhanced magnetic anisotropy could be one of the potential candidates for spin filters.

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