Abstract

Prompt γ-ray spectroscopy of the neutron-rich Kr96, produced in transfer- and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS++ spectrometer. A second excited state, assigned to Jπ=4+, is observed for the first time, and a previously reported level energy of the first 2+ excited state is confirmed. The measured energy ratio R4/2=E(4+)/E(2+)=2.12(1) indicates that this nucleus does not show a well-developed collectivity contrary to that seen in heavier N=60 isotones. This new measurement highlights an abrupt transition of the degree of collectivity as a function of the proton number at Z=36, of similar amplitude to that observed at N=60 at higher Z values. A possible reason for this abrupt transition could be related to the insufficient proton excitations in the g9/2, d5/2, and s1/2 orbitals to generate strong quadrupole correlations or to the coexistence of competing different shapes. An unexpected continuous decrease of R4/2 as a function of the neutron number up to N=60 is also evidenced. This measurement establishes the Kr isotopic chain as the low-Z boundary of the island of deformation for N=60 isotones. A comparison with available theoretical predictions using different beyond mean-field approaches shows that these models fail to reproduce the abrupt transitions at N=60 and Z=36.Received 27 January 2017DOI:https://doi.org/10.1103/PhysRevLett.118.162501Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCollective levelsEnergy levels & level densitiesRare & new isotopesProperties90 ≤ A ≤ 149TechniquesGamma ray spectroscopySpectrometers & spectroscopic techniquesNuclear Physics

Highlights

  • Prompt γ-ray spectroscopy of the neutron-rich 96Kr, produced in transfer- and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS þ þ spectrometer

  • The measured energy ratio R4=2 1⁄4 Eð4þÞ=Eð2þÞ 1⁄4 2.12ð1Þ indicates that this nucleus does not show a well-developed collectivity contrary to that seen in heavier N 1⁄4 60 isotones

  • This new measurement highlights an abrupt transition of the degree of collectivity as a function of the proton number at Z 1⁄4 36, of similar amplitude to that observed at N 1⁄4 60 at higher Z values

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Summary

Introduction

Prompt γ-ray spectroscopy of the neutron-rich 96Kr, produced in transfer- and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS þ þ spectrometer. Calculations support the hypothesis of a quantum phase transition in Zr isotopes [18], and a recent measurement places 97Rb (Z 1⁄4 37) as the cornerstone of this island of deformation [24].

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