Abstract
The Kitaev-Heisenberg (KH) model has been proposed to capture magnetic interactions in iridate Mott insulators on the honeycomb lattice. We show that analogous interactions arise in many other geometries built from edge-sharing IrO${}_{6}$ octahedra, including the pyrochlore and hyperkagome lattices relevant to Ir${}_{2}$O${}_{4}$ and Na${}_{4}$Ir${}_{3}$O${}_{8}$, respectively. The Kitaev spin liquid exact solution does not generalize to these lattices. However, a different, exactly soluble point of the honeycomb lattice KH model, obtained by a four-sublattice transformation to a ferromagnet, generalizes to all of these lattices and even to certain additional further neighbor Heisenberg couplings. A Klein four-group $\ensuremath{\cong}$${\mathbb{Z}}_{2}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{2}$ structure is associated with this mapping (hence Klein duality). A finite lattice admits the duality if a simple geometrical condition is met. This duality predicts fluctuation-free ordered states on these different 2D and 3D lattices, which are analogues of the honeycomb lattice KH stripy order. This result is used in conjunction with a semiclassical Luttinger-Tisza approximation to obtain phase diagrams for KH models on the different lattices. We also discuss a Majorana fermion based mean-field theory at the Kitaev point, which is exact on the honeycomb lattice, for the KH models on the different lattices. We attribute the rich behavior of these models to the interplay of geometric frustration and frustration induced by spin-orbit coupling.
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