Abstract
A kirigami-engineered composite hydrogel membrane is exploited for the construction of three dimensional (3D) solar-tracking evaporator arrays with outstanding evaporation performance and salt tolerance. The hybrid nanofiber network in the hydrogel membrane offers favorable water transport dynamics combined with excellent structural robustness, which are beneficial for the engineering of 3D dynamic structures. Periodic triangular cuts patterned into the membrane allow formation and reconfiguration of 3D conical arrays controlled by uniaxial stretching. With these structures, the tilt angles of the membrane surface are actively tuned to follow the solar trajectory, leading to a solar evaporation rate ~80% higher than that of static planar devices. Furthermore, the tapered 3D flaps and their micro-structured surfaces are capable of localized salt crystallization for prolonged solar desalination, enabling a stable evaporation rate of 3.4 kg m-2 hour-1 even in saturated brine. This versatile design may facilitate the implementation of solar evaporators for desalination and provide inspirations for other soft functional devices with dynamic 3D configurations.
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