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Abstract
The kinetics of oxidation of [Co(NH3)5(NCS)]2+ by peroxodisulphate and periodate were investigated at different ionic strengths, and at different temperatures and concentrations of perchloric acid. Rate constants and activation parameters are also reported in mixed water-organic solvents. It was shown that the acid-base equilibria involving S2O8−2, and IO4− ions are important in the reactions studied. Solvent effects on the oxidation are interpreted in terms of the solvation of both the initial state and the activated complex.
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