Abstract
The reaction kinetics of the HNCO-RAPRENOx process have been studied at temperatures between 1700 and 2500 K in a shock tube equipped with two CW CO probing lasers. The rates of disappearance of NO and formation of CO and H2O products were measured by laser resonance absorption. The reaction was found to be controlled primarily by the rate of the HNCO decomposition reaction which produces the reactive, reducing radical, NH. Addition of NO2 to the system was found to enhance the rates of HNCO disappearance and CO and HNCO reaction via different product channels. H2O production. This effect could be attributed to the enhanced production of NH, OH and NCO by the O +
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