Abstract
HighlightsJanus quasi-solid electrolyte membranes with asymmetric porous structure were constructed, showing a high σLi+ of 1.5 × 10-4 S cm-1 and a high t+ of 0.71.The solvation structures and ion transport dynamics in nanopores have been deciphered, manifesting a concentrated electrolyte-like structure and regulated transport behaviors.Quasi-solid NCM 622||Li cells have been demonstrated to stably cycle for 200 cycles at 1 C, and pouch cell has shown high tolerance for abuse.
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