Janus Carbon Nanotube@poly(butylene adipate-co-terephthalate) Fabric for Stable and Efficient Solar-Driven Interfacial Evaporation.

Abstract

Solar-driven seawater desalination is considered a promising method for alleviating the water crisis worldwide. In recent years, significant efforts have been undertaken to optimize heat management and minimize salt blockage during solar-driven seawater desalination. However, it remains challenging to achieve an efficient and stable seawater evaporator simply and practically. Here, we designed and prepared a novel three-dimensional (3D) water channel evaporator (3D WCE) equipped with a Janus CNT@PBAT fabric (JCPF). The as-prepared Janus CNT@PBAT fabric has broad-band light absorption (∼97.8%), excellent superhydrophobicity (∼162°), and photothermal properties. After optimizing the structure of the thermal insulator, our designed evaporator could realize the equilibrium between enhanced thermal management and sufficient water supply. As a result, the as-prepared evaporator achieved an excellent evaporation rate of 1.576 kg·m-2·h-1 and an energy efficiency of over 92.7% under 1 sun irradiation in 3.5 wt % saline water. Moreover, this evaporator also revealed good salt rejection performance compared to the traditional two-dimensional (2D) water channel evaporator (2D WCE) in high saline water, which could maintain stable evaporation rates under long-term evaporation of 8 h. Our study may develop a simple method for the design and fabrication of a low-cost, effective, and stable solar-driven evaporator for seawater desalination.