Abstract

The effect of 16O→18O isotope substitution on electrical resistivity, magnetoresistance, and ac magnetic susceptibility was studied for La0.35Pr0.35Ca0.3MnO3 epitaxial thin films deposited onto LaAlO3 and SrTiO3 substrates. For the films on LaAlO3, the isotope substitution resulted in the reversible transition from a metal-like to insulating state. The applied magnetic field ( H≥ 2T) transformed the sample with 18O back to the metallic state. The films on SrTiO3 remained metallic at low temperatures for both 16O and 18O, but the shift of the resistivity peak corresponding to onset of metallic state exceeded 63 K after 16O→18O substitution. The temperature dependence of both resistivity and magnetic susceptibility was characterized by hysteresis, especially pronounced in the case of the films on LaAlO3. Such a behavior gives certain indications of the phase separation characteristic of interplay between ferromagnetism and charge ordering.

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