Abstract
Matrix spectroscopy has experienced an enormous development and extension since its invention by Pimentel and Porter. This lecture report is restricted to research carried out in our laboratory concerning various developments in infrared matrix spectroscopy. The main topics are: • classical IR spectroscopy of organic molecules with 7–12 atoms • determination of transferable valence force fields • application of thermal molecular beam-IR matrix spectroscopy for determination of unstable conformers • supersonic molecular beam-IR matrix spectroscopy • linear reactor-IR matrix spectroscopy of complex reaction systems • the problem of molecule-matrix interactions. Typical problems selected from these topics will be illustrated by examples involving mostly polyatomic organic molecules.
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