Abstract
Infrared laser-induced (SF 6) photosensitized decomposition and infrared laser multiphoton decomposition of silacyclopent-3-ene occur as extrusion of silylene, yielding butadiene as a major gaseous product and affording chemical vapour deposition of solid saturated polycarbosilane films. The involvement of H 2Si :, H 2C : and buta-1,3-diene in the formation of the films is revealed through quantification of the gaseous products and identification of H 2Si : and H 2C : by laser induced fluorescence.
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