Ionization dynamics of extended multielectron systems

Abstract

Ionization of multielectron systems is investigated by using one-dimensional, multiconfiguration time-dependent Hartree-Fock calculations. Our analysis reveals the key physical processes underlying ionization of complex systems. The laser-induced multielectron dynamics, and therewith the ionization process, depend on the ratio of laser frequency $({\ensuremath{\omega}}_{0})$ to plasmon frequency $({\ensuremath{\omega}}_{p})$. In the overresonant limit $({\ensuremath{\omega}}_{0}⪢{\ensuremath{\omega}}_{p})$, tunnel ionization is destroyed and ionization takes place by a classical over the barrier mechanism. In the underresonant regime $({\ensuremath{\omega}}_{0}⪡{\ensuremath{\omega}}_{p})$, tunnel ionization remains dominant, but is weakened by a polarization-induced growth of the tunneling barrier.