Abstract
Abnormal “polymer-in-salt” conduction behavior is observed in a solid electrolyte composed of lithium iodide (LiI) and 3-hydroxypropionitrile (HPN). Based on comprehensive investigations by X-ray diffraction (XRD) and Raman and infrared spectroscopy, this abnormal conduction behavior is attributed to the formation of new ionic associates [Li m +I n −]⋯N C ( m > n) and the reinforced hydrogen bonding of I⋯HO in the electrolyte at high LiI concentrations.
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