Abstract
The ion-pair anion efficiency spectrum of Cl − produced in photoexcitations of benzyl chloride is recorded and tentatively assigned as the transitions from the inner-valence molecular orbitals to Rydberg orbitals. Two series transitions 16a′, 6a″ → np ( n = 6, 7, 8, 9, …) are proposed to couple strongly with the ion-pair dissociations in the photon energy range of ca. 14.5–16.0 eV.
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