Abstract

By a comparative analysis of the emission of highly charged ions and energetic electrons the interaction dynamics of intense femtosecond laser fields $({10}^{13}--{10}^{14}\phantom{\rule{0.3em}{0ex}}\mathrm{W}∕{\mathrm{cm}}^{2})$ with nanometer-sized silver clusters is investigated. Using dual laser pulses with variable optical delay the time-dependent cluster response is resolved. A dramatic increase both in the atomic charge state of the ions and the maximum electron kinetic energy is observed for a certain delay of the pulses. Corresponding Vlasov calculations on a metal cluster model system indicate that enhanced cluster ionization as well as the generation of fast electrons coincide with resonant plasmon excitation.

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