Abstract
Two polymorphous compounds with the general formula [Cu(NCS)2(dpk·CH3OH)]n (dpk = di-2-pyridyl-ketone) have been synthesised and have been characterised both structurally and magnetically. The dpk·CH3OH ligand is the result of the metal-promoted solvolysis of dpk in methanol and acts as a neutral donor. X-ray analysis carried out on single crystals for both compounds revealed that compound 1 is dimeric exhibiting double (N,S)-thiocyanate bridges, while com
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