Investigation of the afterpeaks in pulsed microwave argon plasma at atmospheric pressure

Abstract

We studied the energy transport process in pulsed microwave argon plasmas at atmospheric pressure, focusing on the optical emission burst during the pulse-off time called the afterpeak. Guided by experimental observations using nanosecond time resolution imaging and spectroscopic diagnostics, we developed a global simulation model considering time-varying reaction rate coefficients and non-thermal electron energy distribution. Experimental and simulation results show that the afterpeak can be maximized by choosing an appropriate pulse period. Our analysis of the generation and consumption of excited argon species reveals that the rapid drop in electron temperature during the inter-pulse time reduces the diffusive loss of ions and enhances the recombination reactions, which produce the afterpeak. We also reveal that the radiation trapping and high energy level argon must be considered to simulate the afterpeak in atmospheric conditions. The improved understanding of the afterpeak dynamics can be utilized to optimize the power coupling and/or generation of reactive species.