Abstract

Atmospheric pressure plasma jets (APPJs) produce reactive species and electric fields for biomedical applications. Gas shields control plasma plume-surrounding gas interactions, regulating reactive species generation and electric field strength. However, the surface electric field distribution is still unclear and needs urgent attention. Here, the electric field distribution on the surface exposed to a helium APPJ with shielding gas is investigated using the Pockels technique. This study considers the influence of the type of shielding gas (ambient air, dry air, nitrogen, oxygen, nitrogen-oxygen mixture) and the flow rate (2000–6000 sccm). The results show that the surface electric field develops in three phases: establishment, maintenance, and dissipation. Both flow rate and oxygen content of the shielding gas significantly influence surface discharge behavior and the maximum electric field value. The analysis suggests that the establishment phase of the electric field results from charge transfer by ionization waves to the dielectric, while the maintenance of the electric field depends on pulse duration. During the dissipation phase, the positive surface charge attracts negatively charged species to the surface (electrons and negative ions), which causes charge neutralization at the surface. The oxygen content in the shielding gas impacts the electric field establishment phase, with a low oxygen content leading to lower photo-ionization rates and, consequently, surface discharges with branching. Shielding gas flow rates affect the amount of shielding gas mixed into the helium channel. Mixing less oxygen into the APPJ increases the electric field strength, as the ionization potential is lower than nitrogen. Excessive oxygen mixing traps more free electrons due to electronegativity, causing fewer ionized collisions and more negative ions in APPJ, ultimately lowering the electric field strength. This study shows that shielding gas type and flow rates can adjust surface charging, aiding in optimizing biomedical APPJ.

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