Abstract

• Vertical distributions of urban pollution were investigated by instrumented UAVs. • A west-east sampling gradient belt of the built-up area was used for field monitoring. • The concentrations of particulate matter decreased from west to east on Days 2 and 3. • Ground cumulative effects of PM 1 , PM 2.5 and PM 10 were higher than those of SO 2 and NO 2 . Understanding the vertical distribution patterns of air pollution is crucial to elucidate the formation mechanism of extreme air pollution events and explore the air pollution exposure risks of residents. The vertical air pollutant (SO 2 , NO 2 , PM 1 , PM 2.5 and PM 10 ) concentrations along a west-east sampling belt of 0–120 m height were investigated using a multirotor unmanned aerial vehicle (UAV) equipped with mobile sensors on 4 monitoring days. Vertical distribution patterns were explored by ordinary least-squares regression and Pearson correlation coefficient. The results indicated that the concentration of particulate matter decreased gradually from west to the east (S1 to S8) on monitoring Days 2 and 3. The ground cumulative effects of atmospheric particulate matter (PM 1 , PM 2.5 , PM 10 ) were significantly higher than those of gaseous pollutants (SO 2 , NO 2 ). The vertical variation ranges of pollutants from large to small were PM 10 ( k = 0.18), PM 2.5 ( k = 0.16), PM 1 ( k = 0.07), NO 2 ( k = 0.06) and SO 2 ( k = 0.01). Atmospheric particulate matter tends to change significantly with vertical height, and the concentration decreases gradually with increasing height. The proposed UAV based gradient monitoring approach and vertical pollutant change trend analysis method could promote the urban air pollution researches and urban sustainable development.

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