Abstract
A series of polymetallic complexes are being developed for use in converting solar radiation to usable chemical potential energy. The system is made up of three components: 1) A highly-absorbing (antenna) metal center which absorbs visible light but is photochemically unreactive; 2) A second metal center which undergoes a useful chemical reaction from a non-spectroscopic excited state; and 3) A bridging ligand which couples the two metal fragments and facilitates intramolecular energy transfer from the antenna to the reactive fragment. This paper will focus on optimizing the three components of the system.
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