Abstract
A major assumption in the Rice--Ramsberger--Cassel--Marcus theory (RRCM theory) is that the states of an activated molecule are filled with equal probability [i, 2]. In a real molecule, the transitions in general are not equally probable, so it is of interest to examine deviations from the RRCM model. This is necessary particularly in order to set up any theory that incorporates explicitly the detailed energy redistribution in an active molecule.
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