Intracavity spectroscopy with modulated multimode lasers

Abstract

The output of a cw multimode dye laser with an intracavity narrow-band absorber and its pump power modulated shows spectral condensation on both wings of the absorption line. This indicates phase locking of two groups of laser modes. The dispersion of the absorber modifies the mode spacing of the laser such that mode groups on both sides of the absorption line get into resonance with the modulation. These mode groups feel smaller loss and acquire the total laser power. Spectra of the laser output reveal the total absorption coefficient, the homogeneous broadening of the absorber, and the spectral width of individual laser modes.