Interplay of charge and spin fluctuations of strongly interacting electrons on the kagome lattice

Abstract

We study electrons hopping on a kagome lattice at third filling described by an extended Hubbard Hamiltonian with on-site and nearest-neighbor repulsions in the strongly correlated limit. As a consequence of the commensurate filling and the large interactions, each triangle has precisely two electrons in the effective low-energy description, and these electrons form chains of different lengths. The effective Hamiltonian includes the ring exchange around the hexagons as well as the nearest-neighbor Heisenberg interaction. Using large-scale exact diagonalization, we find that the effective model exhibits two phases: If the charge fluctuations are small, the magnetic fluctuations confine the charges to short loops around hexagons, yielding a gapped charge-ordered phase. When the charge fluctuations dominate, the system undergoes a quantum phase transition to a resonating plaquette phase with ordered spins and gapless spin excitations. We find that a peculiar conservation law is fulfilled: the electron in the chains can be divided into two sublattices, and this division is conserved by the ring exchange term.