Abstract

The magnetic field-induced changes in the conductivity of metals are the subject of intense interest, both for revealing new phenomena and as a valuable tool for determining their Fermi surface. Here we report a hitherto unobserved magnetoresistive effect in ultra-clean layered metals, namely a negative longitudinal magnetoresistance that is capable of overcoming their very pronounced orbital one. This effect is correlated with the interlayer coupling disappearing for fields applied along the so-called Yamaji angles where the interlayer coupling vanishes. Therefore, it is intrinsically associated with the Fermi points in the field-induced quasi-one-dimensional electronic dispersion, implying that it results from the axial anomaly among these Fermi points. In its original formulation, the anomaly is predicted to violate separate number conservation laws for left- and right-handed chiral (for example, Weyl) fermions. Its observation in PdCoO2, PtCoO2 and Sr2RuO4 suggests that the anomaly affects the transport of clean conductors, in particular near the quantum limit.

Highlights

  • The magnetic field-induced changes in the conductivity of metals are the subject of intense interest, both for revealing new phenomena and as a valuable tool for determining their Fermi surface

  • For the correlated Sr2RuO4, the longitudinal negative magnetoresistivity effect is observable but only in the cleanest samples, that is, those displaying the highest superconducting transition temperatures. We suggest that this effect might result from the axial anomaly between Fermi points in a field-induced, quasi-one-dimensional electronic dispersion

  • Negative magnetoresistivity is a common feature of ferromagnetic metals near their Curie temperature, or of samples having dimensions comparable to their electronic mean free path where the winding of the electronic orbits under a magnetic field reduces the scattering from the surface

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Summary

Introduction

The magnetic field-induced changes in the conductivity of metals are the subject of intense interest, both for revealing new phenomena and as a valuable tool for determining their Fermi surface. A series of compounds were proposed to be candidate Weyl semi-metals characterized by a linear touching between the valence and the conduction bands at several points (Weyl points) of their Brillouin zone[8] These Weyl points are predicted to lead to a pronounced negative magnetoresistivity for electric fields aligned along a magnetic field due to the so-called axial anomaly[9,10]. For the correlated Sr2RuO4, the longitudinal negative magnetoresistivity effect is observable but only in the cleanest samples, that is, those displaying the highest superconducting transition temperatures We suggest that this effect might result from the axial anomaly between Fermi points in a field-induced, quasi-one-dimensional electronic dispersion

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