Abstract
The 266 nm photodissociation of gaseous C 6H 5NO has been studied by monitoring the nascent NO ( X 2Π v″=0–3 ) product using the single-photon laser-induced fluorescence technique. The rotational-state distributions of the nascent NO photofragment have been measured and can be characterized by Bolzmann temperatures. The vibrational-state and Λ-doublet populations were also determined. Energy disposal into the internal degrees of freedom of NO ( X 2Π ) photofragment is about 18% of the total available energy. Some planarity in the fragmentation process was observed.
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