Abstract
Temperature-dependent molecular dynamics of CS 2 liquid are examined in femtosecond time-resolved impulsive stimulated scattering experiments. At temperatures T⩽ 240 K, weakly oscillatory time-dependent responses are observed. These are interpreted in terms of librations of molecules about their local potential minima. The librations undergo rapid inhomogeneous dephasing. Temperature-dependent values of the configuration-averaged librational frequency and the extent of inhomogeneity in that frequency are determined.
Full Text 
Sign-in/Register to access full text options
Sign-in/Register to access full text options 
Paper version not known
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a call
