Abstract
AbstractAs a basis for the design of electroactive materials, mono‐ and bis‐tetrathiafulvalene (TTF) derivatives with one and two amide units were prepared to investigate how hydrogen bonding induces electronic communication. The bis‐TTF compound exhibited a mixed‐valence state as a result of electronic interactions among the TTF units. Comparison with non‐hydrogen‐bonding N‐methylated analogues indicated that the electronic interaction observed occurs between intermolecular TTF units owing to the formation of supramolecular assemblies induced by hydrogen bonds.
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