Abstract

Abstract Femtosecond laser interactions inside transparent dielectric films of refractive index, n film, with tight focusing presents strong nonlinear interactions that can be preferentially confined at the fringe maxima as formed by Fabry-Perot interference, to generate thin nanoscale plasma disks separated on half-wavelength, λ/2n film. The nano-thin disk explosions can be controlled inside the film to cleave open subwavelength internal cavities at single or multiple periodic depths at low laser exposure, while higher exposure will eject a quantised number of film segments with segment thickness defined by the laser wavelength. This new method enables high-resolution film patterning for ejecting nanodisks at quantised film depth for colouring and three-dimensional (3D) surface structuring, as well as for fabrication of free-standing nanofilms.

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