Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect

Abstract

We demonstrate that the optical linewidth of Rydberg excitons in Cu2O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical and modes. The consequences for the observation of polariton effects are discussed. We find that an anti-crossing of photon and exciton dispersions exists only for states with main quantum numbers n > 28, so polariton effects do not play any role in the experiments reported up to now.