Integrated Perovskite/Organic Photovoltaics with Ultrahigh Photocurrent and Photoresponse Approaching 1000 nm

Abstract

To enhance the photoresponse of commonly used perovskite materials in the near‐infrared (NIR) region, a fused‐ring electron acceptor (F8IC) with strong NIR absorption and high electron mobility is used to blend with a narrow‐bandgap polymer donor (PTB7‐Th) to construct an organic bulk heterojunction (OBHJ), and this OBHJ is then integrated with the perovskite solar cells (PSCs). The integrated perovskite/OBHJ solar cells exhibit a strong photoresponse approaching 1000 nm and an ultrahigh short‐circuit current density of 28.2 mA cm−2, which is much higher than that of traditional PSCs and organic solar cells.