Abstract

Water oxidation is a key reaction in natural and artificial photosynthesis. In their Research Article on page 5965, Mio Kondo, Shigeyuki Masaoka, and co-workers report a facile strategy to integrate catalytic centers and hole transporters in one system, which is inspired by the natural water oxidation catalyst. A metal-complex-based precursor was electrochemically polymerized, and the obtained polymer-based material exhibits excellent hole-transporting ability and catalyzes water oxidation with high performance.

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