Abstract

With the increasing application of global navigation satellite system (GNSS) technology in the field of meteorology, satellite-derived zenith tropospheric delay (ZTD) and precipitable water vapor (PWV) data have been used to explore the spatial coverage pattern of PM2.5 concentrations. In this study, the PM2.5 concentration data obtained from 340 PM2.5 ground stations in south-central China were used to analyze the variation patterns of PM2.5 in south-central China at different time periods, and six PM2.5 interpolation models were developed in the region. The spatial and temporal PM2.5 variation patterns in central and southern China were analyzed from the perspectives of time series variations and spatial distribution characteristics, and six types of interpolation models were established in central and southern China. (1) Through correlation analysis, and exploratory regression and geographical detector methods, the correlation analysis of PM2.5-related variables showed that the GNSS-derived PWV and ZTD were negatively correlated with PM2.5, and that their significances and contributions to the spatial analysis were good. (2) Three types of suitable variable combinations were selected for modeling through a collinearity diagnosis, and six types of models (geographically weighted regression (GWR), geographically weighted regression kriging (GWRK), geographically weighted regression—empirical bayesian kriging (GWR-EBK), multiscale geographically weighted regression (MGWR), multiscale geographically weighted regression kriging (MGWRK), and multiscale geographically weighted regression—empirical bayesian kriging (MGWR-EBK)) were constructed. The overall R2 of the GWR-EBK model construction was the best (annual: 0.962, winter: 0.966, spring: 0.926, summer: 0.873, and autumn: 0.908), and the interpolation accuracy of the GWR-EBK model constructed by inputting ZTD was the best overall, with an average RMSE of 3.22 μg/m3 recorded, while the GWR-EBK model constructed by inputting PWV had the highest interpolation accuracy in winter, with an RMSE of 4.5 μg/m3 recorded; these values were 2.17% and 4.26% higher than the RMSE values of the other two types of models (ZTD and temperature) in winter, respectively. (3) The introduction of the empirical Bayesian kriging method to interpolate the residuals of the models (GWR and MGWR) and to then correct the original interpolation results of the models was the most effective, and the accuracy improvement percentage was better than that of the ordinary kriging method. The average improvement ratios of the GWRK and GWR-EBK models compared with that of the GWR model were 5.04% and 14.74%, respectively, and the average improvement ratios of the MGWRK and MGWR-EBK models compared with that of the MGWR model were 2.79% and 12.66%, respectively. (4) Elevation intervals and provinces were classified, and the influence of the elevation and the spatial distribution of the plane on the accuracy of the PM2.5 regional model was discussed. The experiments showed that the accuracy of the constructed regional model decreased as the elevation increased. The accuracies of the models in representing Henan, Hubei and Hunan provinces were lower than those of the models in representing Guangdong and Guangxi provinces.

Highlights

  • PM2.5 refers to fine particulate matter with a diameter of less than or equal to 2.5 μm existing in the ambient air; this matter has the characteristics of a long suspension time in the air, a long transportation distance, strong activity, and easy absorption of toxic and harmful substances; especially high PM2.5 concentrations cause occurrences of hazy weather [1,2,3]

  • Note: DEM means the elevation values obtained from the digital elevation model, WIN means wind, PRE means pressure, TEM means temperature, ZTD means zenith tropospheric delay, PWV means precipitable water vapor, GNSS means global navigation satellite system

  • Compared with the interpolation effect of a single geographically weighted regression-type model for PM2.5, the combined model shows a stronger advantage, and the overall best performance in this area is obtained with the Geographically Weighted Regression—Empirical Bayesian Kriging (GWR-EBK) model, indicating that the empirical Bayesian kriging method is better for the explanation and interpretation of GWR residuals; further, the GWR-EBK model can improve the accuracy by 14.74% more than the GWR model

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Summary

Introduction

PM2.5 refers to fine particulate matter with a diameter of less than or equal to 2.5 μm existing in the ambient air; this matter has the characteristics of a long suspension time in the air, a long transportation distance, strong activity, and easy absorption of toxic and harmful substances; especially high PM2.5 concentrations cause occurrences of hazy weather [1,2,3]. Since 2012, China has built a large number of ground-based PM2.5 stations nationwide. China is a vast country, and the number of ground-based. PM2.5 stations is still scarce, and they cannot accurately explain all the temporal and spatial characteristics of PM2.5 , limiting the application of PM2.5 data in a variety of practical applications. It is necessary to further study how to obtain continuous and accurate regional PM2.5 distributions on different temporal and spatial scales and how to use limited station-derived data to conduct high-precision regional PM2.5 temporal and spatial interpolations, and these applications have become a research hotspot. China is a vast country, and many scholars have tried to explore the variation patterns of PM2.5 in different regions of China, such as North China [4], the Yangtze River Economic

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