Abstract
The infra-red spectrum of NSCl was studied from 300 to 4000 cm −1. The two fundamentals v 1 and v 2 were directly observed and the third one v 3 was calculated from the overtone and combination bands. It was confirmed that NSCl has the structure NSCl with C s-symmetry and not SNCl. Force constants, mean amplitudes of vibration, molar thermo-dynamic functions and molecular polarizability were computed and the results briefly discussed.
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