Influence of specific energy inhomogeneity on the CO2 splitting performance in a high-power plasma jet

Abstract

Plasma-based CO2 conversion is a promising pathway towards greenhouse gas recycling. In the corresponding research field, various types of plasma reactors are applied for carbon dioxide dissociation. So far, spatial inhomogeneities of the specific energy (SEI) distribution in plasma generators, e.g., induced by non-uniform heating or an inhomogeneous mass distribution, are not the focus of the investigations. In this work, the spatial inhomogeneity of mass-specific enthalpy in the plasma jet of the inductive plasma generator IPG4 at the Institute of Space Systems (IRS) is examined. For this purpose, the mean mass-specific enthalpy as well as the radial distribution of the local enthalpy are measured using plasma probes. Moreover, the influence of the determined specific enthalpy inhomogeneity on the CO2 splitting performance is quantified. It is shown that an inhomogeneous radial distribution of the specific energy can significantly lower the carbon dioxide conversion, compared to a homogeneous case. With regards to IPG4, the performance reduction is 16%.