Abstract

The influence of pressure on the gas/liquid interfacial area is investigated in the pressure range of 0.2–0.3 MPa by using a tray column test rig. A simulated waste gas, which consisted of 30% CO2 and 70% air, was used in this study. Distilled water was employed as an absorbent. The temperature of the inlet water was 19 °C. The inlet volumetric flow rate of water was 0.17 m3/h. Two series of experiments were performed; the first series was performed at inlet gas flow rate 15 Nm3/h, whereas the second series was at 20 Nm3/h of inlet gas flow rate. The results showed that the gas/liquid interfacial area decreases when the total pressure is increased. The effect of pressure on the gas/liquid interfacial area at high inlet volumetric gas flow rates is more significant than at low inlet volumetric gas flow rates. The authors studied the effect of decreasing the interfacial area on the performance of a tray column for CO2 capture.

Highlights

  • The global atmospheric concentration of carbon dioxide and its contribution to global warming requires technical measures to limit the emission of this greenhouse gas

  • The results showed that the gas/liquid interfacial area decreases when the total pressure is increased

  • Barzagli et al (2014) [3] studied nonaqueous amine solvents such as 2-(isopropylamino)ethanol (IPMEA), 2-(tert-butylamino)ethanol (TBMEA) and N-methyl-2,2’-iminodiethanol(MDEA) for CO2 capture and found that CO2 removal efficiency was in the range of 87–95% at equilibrium, depending on the operational conditions

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Summary

Introduction

The global atmospheric concentration of carbon dioxide and its contribution to global warming requires technical measures to limit the emission of this greenhouse gas. One possibility is by separating the carbon dioxide from the waste gas stream of fossil power plants by applying absorption technologies. The absorption process of CO2 can be performed using solvents with different additives. Amine solvents such as monoethanolamine (MEA), diethanolamine (DEA), and methyldiethanolamine (MDEA) are common for CO2 capture (Wilk et al 2017) [1]. Barzagli et al (2014) [3] studied nonaqueous amine solvents such as 2-(isopropylamino)ethanol (IPMEA), 2-(tert-butylamino)ethanol (TBMEA) and N-methyl-2,2’-iminodiethanol(MDEA) for CO2 capture and found that CO2 removal efficiency was in the range of 87–95% at equilibrium, depending on the operational conditions. The absorbent enters the absorber from the top, and the waste gas, which contains

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